Vol. 32, issue 06, article # 1

Sakerin S. M., Golobokova L. P., Kabanov D. M., Kalashnikova D. A., Kozlov V. S., Kruglinsky I. A., Makarov V. I., Makshtas A. P., Popova S. A., Radionov V. F., Simonova G. V., Turchinovich Yu. S., Khodzher T. V., Khuriganova O. I., Chankina O. V., Chernov D. G. Measurements of physical-chemical characteristics of atmospheric aerosol at “Ice Base Cape Baranov” in 2018. // Optika Atmosfery i Okeana. 2019. V. 32. No. 06. P. 421–429. DOI: 10.15372/AOO20190601 [in Russian].
Copy the reference to clipboard

Abstract:

We discuss the results of measurements in the region of Cape Baranov (the Severnaya Zemlya archipelago) of the set of physical-chemical characteristics of atmospheric aerosol: aerosol optical depth, aerosol and black carbon concentrations, elemental and ion composition of aerosol, organic and elemental carbon contents in aerosol, and isotopic composition of carbon in the aerosol and snow samples. It is shown that the average values of the most aerosol characteristics, measured in April–June 2018, are much lower than in the Arctic settlement Barentsburg (Spitsbergen archipelago) and several-fold smaller than in the south of Western Siberia in the same period of time.

Keywords:

aerosol, black carbon, ionic, elemental, isotopic composition, Northern Earth

References:

1. Barteneva O.D., Nikitinskaya N.I., Sakunov G.G., Veselova L.K. Prozrachnost' tolshchi atmosfery v vidimoj i blizhnej IK-oblasti spektra. L.: Gidrometeoizdat, 1991. 224 p.
2. Tomasi C., Kokhanovsky A.A., Lupi A., Ritter C., Smirnov A., Mazzola M., Stone R.S., Lanconelli C., Vitale V., Holben B.N., Nyeki S., Wehrli C., Altonen V., de Leeuw G., Rodriguez E., Herber A.B., Stebel K., Stohl A., ONeill N.T., Radionov V.F., Zielinski T., Petelski T., Sakerin S.M., Kabanov D.M., Xue Y., Mei L., Istomina L., Wagener R., McArthur B., Sobolewski P.S., Butler J., Kivi R., Courcoux Y., Larouche P., Broccardo S., Piketh S.J. Aerosol remote sensing in polar regions // Earth-Sci. Rev. 2015. V. 140. P. 108–157. URL: http://dx.doi.org/10.1016/j.earscirev.2014.11.001.
3. Shevchenko V.P., Lisitsyn A.P., Vinogradova A.A., Smirnov V.V., Serova V.V., Shtajn R. Aerozoli Arktiki – rezul'taty desyatiletnikh issledovanij // Optika atmosf. i okeana. 2000. V. 13, N 6–7. P. 551–576.
4. Shevchenko V.P., Vinogradova A.A., Lisitsyn A.P., Navigatskij A.N., Goryunova N.V. Atmosfernyye aerozoli kak istochnik osadochnogo veshchestva i zagryaznenij v Severnom Ledovitom okeane // Sistema morya Laptevykh i prilegayushchikh morej Arktiki: sovremennoye sostoyaniye i istoriya razvitiya. M.: Izd-vo Mosk. un-ta, 2009. P. 150–172.
5. Eleftheriadis K., Vratolis S., Nyeki S. Aerosol black carbon in the European Arctic: Measurements at Zeppelin station, Ny-Ålesund, Svalbard from 1998–2007 // Geophys. Res. Let. 2009. V. 36. DOI: 10.1029/2008GL035741.
6. Sakerin S.M., Chernov D.G., Kabanov D.M., Kozlov V.S., Panchenko M.V., Pol'kin V.V., Radionov V.F. Predvaritel'nyye rezul'taty issledovanij aerozol'nykh kharakteristik atmosfery v rajone Barentsburga (Shpitsbergen) // Problemy Arktiki i Antarktiki. 2012. N 1(91). P. 20–31.
7. Stone R.S., Sharma S., Herber A., Eleftheriadis K., Nelson D.W. A characterization of Arctic aerosols on the basis of aerosol optical depth and black carbon measurements // Elem. Sci. Anth. 2014. V. 2. 27 p. DOI: 10.12952/journal.elementa.000027.
8. Schmeisser L., Backman J., Ogren J.A., Andrews E., Asmi E., Starkweather S., Uttal T., Fiebig M., Sharma S., Eleftheriadis K., Vratolis S., Bergin M., Tunved P., Jefferson A. Seasonality of aerosol optical properties in the Arctic // Atmos. Chem. Phys. 2018. V. 18, N 16. P. 11599–11622.
9. Shevchenko V.P., Starodymova D.P., Vinogradova A.A., Lisitsyn A.P., Makarov V.N., Popova S.A., Sivonen V.V., Sivonen V.P. Elementnyj i organicheskij uglerod v atmosfernom aerozole nad severo-zapadnym poberezh'yem Kandalakshskogo zaliva Belogo morya // Dokl. RAN. 2015. V. 461, N 1. P. 70–74.
10. Singh D.K., Kawamura K., Yanase A., Barrie L.A. Distributions of polycyclic aromatic hydrocarbons, aromatic ketones, carboxylic acids, and trace metals in Arctic aerosols: Long-range atmospheric transport, photochemical degradation/production at polar sunrise // Environ. Sci. Technol. 2017. V. 51. Р. 8992−9004. DOI: 10.1021/acs.est.7b01644.
11. Lange R., DallOsto M., Skov H., Nøjgaard J.K., Nielsen I.E., Beddows D.C.S., Simo R., Harrison R.M., Massling A. Characterization of distinct Arctic aerosol accumulation modes and theirsources // Atmos. Environ. 2018. V. 183. Р. 1–10. URL: https://doi.org/10.1016/j.atmosenv.2018.03.060.
12. Popovicheva О., Diapouli E., Makshtas A., Shonija N., Manousakas M., Saraga D., Uttal T., Eleftheriadis K. East Siberian Arctic background and black carbon polluted aerosols at HMO Tiksi // Sci. Total Environ. 2019. V. 655. P. 924–938. URL: https://doi.org/10.1016/j.scitotenv.2018.11.165.
13. Widory D. Combustibles, fuels and their combustion products: A view through carbon isotopes // Combust. Theory Modell. 2006. V. 10. P. 831–841.
14. Vinogradova A.A., Ponomareva T.Ya. Atmosfernyj perenos antropogennykh primesej v arkticheskiye rajony Russia (1986–2010) // Optika atmosf. i okeana. 2012. V. 25, N 6. P. 475–483; Vinogradovа А.А., Pоnоmаrevа Т.Ya. Atmospheric transport of anthropogenic impurities to the Russian arctic (1986–2010) // Atmos. Ocean. Opt. 2012. V. 25, N 6. P. 414–422.
15. Vinogradova A.A., Smirnov N.S., Korotkov V.N., Romanovskaya A.A. Lesnyye pozhary v Sibiri i na Dal'nem Vostoke: emissii i atmosfernyj perenos chernogo ugleroda v Arktiku // Optika atmosf. i okeana. 2015. V. 28, N 6. P. 512–520. DOI: 10.15372/AOO20150603; Vinogradovа А.А., Smirnov N.S., Korotkov V.N., Rоmanovskaya А.А. Forest fires in Siberia and the Far East: Emissions and atmospheric transport of black carbon to the Arctic // Atmos. Ocean. Opt. 2015. V. 28, N 6. P. 566–574.
16. Vinogradova A.A., Vasil'yeva A.V. Chernyj uglerod v vozdukhe severnykh rajonov Rossii: istochniki, prostranstvennyye i vremennyye variatsii // Optika atmosf. i okeana. 2017. V. 30, N 6. P. 467–475; Vinogradovа А.А., Vasilevа А.V. Black carbon in air over northern regions of Russia: Sources and spatiotemporal variations // Atmos. Ocean. Opt. 2017. V. 30, N 6. P. 533–541.
17. Makshtas A.P., Uttal T. Nachalo sovmestnykh Rossijsko-amerikanskikh atmosfernykh nablyudenij v Tiksi // Ros. polyar. issled. 2010. N 2. P. 35–38.
18. Asmi E., Kondratyev V., Brus D., Laurila T., Lihavainen H., Backman J., Vakkari V., Aurela M., Hatakka J., Viisanen Y., Uttal T., Ivakhov V., Makshtas A. Aerosol size distribution seasonal characteristics measured in Tiksi, Russian Arctic // Atmos. Chem. Phys. 2016. V. 16. P. 1271–1287. DOI: 10.5194/acp-16-1271-2016.
19. Makshtas A.P., Sokolov V.T. Nauchno-issledovatel'skij statsionar «Ledovaya baza “Mys Baranova”» – letnij polevoj sezon 2014 year. // Ros. polyar. issled. 2014. N 3(17). P. 10–12.
20. Sakerin S.M., Bobrikov A.A., Bukin O.A., Golobokova L.P., Polkin Vas.V., Polkin Vik.V., Shmirko K.A., Kabanov D.M., Khodzher T.V., Onischuk N.A., Pavlov A.N., Potemkin V.L., Radionov V.F. On measurements of aerosol-gas composition of the atmosphere during two expeditions in 2013 along Northern Sea Route // Atmos. Chem. Phys. 2015. V. 15, iss. 21. P. 12413–12443. DOI: 10.5194/acp-15-1-2015.
21. Popovicheva O.B., Evangeliou N., Eleftheriadis K, Kalogridis A.C., Sitnikov N., Eckhard S., Stohl A. Black carbon sources constrained by observations in the Russian High Arctic // Environ. Sci. Technol. 2017. V. 51, N 7. P. 3871–3879. DOI: 10.1021/acs.est.6b05832.
22. Sakerin S.M., Kabanov D.M., Pol’kin V.V., Golobokova L.P., Zenkova P.N., Kessel A.S., Pol’kin Vas.V., Radionov V.F., Terpugova S.A., Urazgildeeva A.V., Khodzher T.V., Khuriganowa O.I. Features of spatial distribution of aerosol characteristics over Arctic seas // Proc. SPIE. 2018. V. 10833, N 39. DOI: 10.1117/12.2502013.
23. Antokhina O.Yu., Antokhin P.N., Arshinova V.G., Arshinov M.Yu., Belan B.D., Belan S.B., Davydov D.K., Ivlev G.A., Kozlov A.V., Nédélec Ph., Paris J.-D., Rasskazchikova T.M., Savkin D.Ye., Simonenkov D.V., Sklyadneva T.K., Tolmachev G.N., Fofonov A.V. Vertikal'noye raspredeleniye gazovykh i aerozol'nykh primesej vozdukha nad rossijskim sektorom Arktiki // Optika atmosf. i okeana. 2017. V. 30, N 12. P. 1043–1052; Antokhina О.Yu., Antokhin P.N., Аrshinovа V.G., Аrshinov М.Yu., Bеlan B.D., Bеlan S.B., Dаvydov D.K., Ivlev G.А., Kоzlov А.V., Nédélec Ph., Paris J.-D., Rasskаzchikova Т.М., Sаvkin D.Е., Simonenkov D.V., Sklyadnevа Т.K., Тоlmachev G.N., Fоfonov А.V. Vertical distributions of gaseous and aerosol admixtures in air over the Russian Arctic // Atmos. Ocean. Opt. 2018. V. 31, N 3. P. 300–310.
24. Kirin D.V., Krutikov N.O., Luk'yanov A.N., Strunin A.M., Strunin M.A. Rezul'taty sravnitel'nogo analiza rasprostraneniya aerozol'nykh primesej v atmosfere regionov Arktiki i Moskovskoj oblasti po dannym samoletnykh issledovanij v 2014–2015 years // Tr. Voyen.-kosm. akad. im. A.F. Mozhajskogo. 2018. Iss. 662. P. 219–223.
25. Stohl A., Andrews E., Burkhart J.F., Forster C., Herber A., Hoch S.W., Kowal D., Lunder C., Mefford T., Ogren J.A., Sharma S., Spichtinger N., Stebel K., Stone R., Ström J., Tørseth K., Wehrli C., Yttri K.E. Pan-Arctic enhancements of light absorbing aerosol concentrations due to North American boreal forest fires during summer 2004 // J. Geophys. Res. 2006. V. 111, N D22214. DOI: 10.1029/2006JD007216.
26. Eck T.F., Holben B.N., Reid J.S., Sinyuk A., Hyer E.J., O’Neill N.T., Shaw G.E., Vande Castle J.R., Chapin F.S., Dubovik O., Smirnov A., Vermote E., Schafer J.S., Giles D., Slutsker I., Sorokine M., Newcomb W.W. Optical properties of boreal region biomass burning aerosols in central Alaska and seasonal variation of aerosol optical depth at an Arctic coastal site // J. Geophys. Res. 2009. V. 114, N D11201. DOI: 10.1029/2008JD010870.
27. Sakerin S.M., Kabanov D.M., Radionov V.F., Chernov D.G., Turchinovich Yu.S., Lubo-Lesnichenko K.Ye., Prakhov A.N. Obobshcheniye rezul'tatov izmerenij spektral'noj aerozol'noj opticheskoj tolshchiny atmosfery na arkh. Shpitsbergen v 2011–2016 years. // Optika atmosf. i okeana. 2017. V. 30, N 11. P. 948–955. DOI: 10.15372/AOO20171107; Sаkerin S.М., Kаbаnov D.М., Rаdionov V.F., Chernov D.G., Turchinovich Yu.S., Lubо-Lesnichenko K.Е., Prakhov А.N. Generalization of results of atmospheric aerosol optical depth measurements on Spitsbergen Archipelago in 2011–2016 // Atmos. Ocean. Opt. 2018. V. 31, N 2. P. 163–170.
28. Vinogradova A.A., Titkova T.B., Ivanova Yu.A. Epizody anomal'no vysokoj kontsentratsii chernogo ugleroda v prizemnom vozdukhe v rajone stantsii Tiksi, Yakutiya // Optika atmosf. i okeana. 2018. V. 31, N 10. P. 837–844. DOI: 10.15372/AOO20181010; Vinogradovа А.А., Тitkova Т.B., Ivanovа Yu.А. Episodes with anomalously high black carbon concentration in surface air in the Region of Tiksi Station, Yakutiya // Atmos. Ocean. Opt. 2019. V. 32, N 1. P. 94–102.
29. Golobokova L.P., Pol'kin V.V., Onishchuk N.A., Khuriganova O.I., Tikhomirov A.B., Terpugova S.A., Pol'kin Vas.V., Turchinovich Yu.S., Radionov V.F. Izmenchivost' khimicheskogo sostava aerozolya v prizemnom sloye atmosfery perekhodnoj zony «materik–okean» v rajone Vostochnoj Antarktidy // Led i sneg. 2016. V. 56, N 2. P. 177–188.
30. Makarov V.I., Koutsenogii K.P., Koutsenogii P.K. Daily and seasonal changes of organic and inorganic carbon content in atmospheric aerosol Novosibirsk region // J. Aerosol Sci. 1999. V. 30. P. S255–S256.
31. Piminov P.A., Baranov G.N., Bogomyagkov A.V., Berkaev D.E., Borin V.M., Dorokhov V.L., Karnaev S.E., Kiselev V.A., Levichev E.B., Meshkov O.I., Mishnev S.I., Nikitin S.A., Nikolaev I.B., Sinyatkin S.V., Vobly P.D., Zolotarev K.V., Zhuravlev A.N. Synchrotron radiation research and application at VEPP-4 // Phys. Proc. 2016. V. 84. Р. 19–26. DOI: 10.1016/j.phpro.2016.11.005.
32. Kulipanov G.N., Mezentsev N.A., Pindyurin V.F. Synchrotron radiation in Novosibirsk: The first 13 years // J. Struct. Chem. 2016. V. 57, N 7. Р. 1277–1287. DOI: 10.1134/S0022476616070015.
33. Lebedev A.T. Mass-spektrometriya dlya analiza ob"yektov okruzhayushchej sredy. M.: Tefnosfera, 2013. 632 p.
34. Simonova G., Volkov Yu., Kozlov V., Shmargunov V., Kalashnikova D. Atmospheric air pollution studies using the isotope mass-spectrometry // 18th Intern. Multidisciplinary Scientific GeoConference SGEM 2018: Conf. Proc. Bulgaria. 2018. V. 18, iss. 4.2. P. 343–348. DOI: 10/5593/sgem2018/4.2.
35. Radionov V.F., Kabanov D.M., Kozlov V.V., Sakerin S.M., Sidorova O.R., Chernov D.G. Opticheskiye i mikrofizicheskiye kharakteristiki aerozolya v rajone Barentsburga (2011–2017) // Kompleksnyye issledovaniya prirody Shpitsbergena i prilegayushchego shel'fa: Tez. dokl. XIV Vseros. nauch. konf. s mezhdunar. uchastiyem (Murmansk, 30 october – 2 november 2018 year.). Апатиты: Изд-во ФИЦ КНЦ РАН, 2018. 133 с. DOI: 10.25702/KSC.978.5.91137.374.0.
36. Kozlov V.S., Panchenko M.V., Shmargunov V.P., Chernov D.G., Yausheva E.P., Pol’kin V.V., Terpugova S.A. Long-term investigations of the spatiotemporal variability of Black Carbon and aerosol concentrations in the troposphere of West Siberia and Russian Subarctic // Chemistry for Sustainable Development. 2016. V. 24, N 4. P. 423–440.
37. Xie Y.-L., Hopke P.K., Paatero P., Barrie L.A., Li S.-M. Identification of source nature and seasonal variations of arctic aerosol by positive matrix factorization // J. Atmos. Sci. 1999. V. 56. Р. 240–260.
38. Oyabu I., Matoba S., Yamasaki T., Kadota M., Iizuka Y. Seasonal variations in the major chemical species of snow at the South East Dome in Greenland // Polar Sci. 2016. V. 10. P. 36–42.
39. Pempkowiak J., Zieliński T., Petelski T., Zaborska A., Bełdowski J. Recent alterations of aerosol concentration, mercury distribution and organic matter deposition in the Arctic // Papers on Global Change. 2011. V. 18. P. 23–33.
40. Parker B.C., Zeller E.J., Gow A.J. Nitrogenous chemical composition of Antarcticice and snow // Antarctic J. US. 1982. V. 14, N 5. Р. 80–82.
41. Keene W.C., Khalil M.A.K., Erickson III D.J., McCulloch A., Graedel T.E., Lobert J.M., Aucott M.L., Gong S.L., Harper D.B., Kleiman G., Midgley P., Moore R.M., Seuzaret C., Sturges W.T., Benkovitz C.M., Koropalov V., Barrie L.A., Li Y.F. Composite global emissions of reactive chlorine from anthropogenic and natural sources: Reactive Chlorine Emissions Inventory // J. Geophys. Res. Atmos. D. 1999. V. 104, N 7. P. 8429–8440. DOI: 10.1029/1998JD100084.
42. Cabada J.C., Pandis S.N., Subramanian R., Robinson A.L., Polidori A., Turpin B. Estimating the secondary organic aerosol contribution to PM2.5 using the EC tracer method // Aerosp. Sci. Technol. 2004. V. 38. P. 140–155. DOI: 10.1080/02786820390229084.
43. Winiger P., Andersson A., Eckhardt S., Stohl A., Gustafsson Ö. The sources of atmospheric black carbon at a European gateway to the Arctic // Nat. Commun. 2016. N 12776. DOI: 10.1038/ncomms12776/www.nature.com/naturecommunications.