Vol. 39, issue 08, article # 7

Firsov K. M., Chesnokova T. Yu., Razmolov A. A. Behavior features of the CO2 and CH4 longwave radiative forcing in the atmosphere of Western Siberia. // Optika Atmosfery i Okeana. 2026. V. 39. No. 08. P. 689–698. DOI: 10.15372/AOO20260807 [in Russian].
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Abstract:

Observed growth of the atmospheric concentration of gases, such as CO2 and CH4, strengthens the greenhouse effect in the atmosphere and impacts on climate. One of the characteristics of the greenhouse effect is the radiative forcing of the atmospheric gases which is defined as the difference between the longwave radiative fluxes at different concentrations of gases other parameters of the atmosphere being constant. From 1990 to 2023, the radiative forcing of long-lived greenhouse gases due to their concentration grow from the pre-industrial period (1750 year) has increased by more than 50%. In the work, the impact of atmospheric water vapor content variability on the CO2 and CH4 radiative forcing for summer and winter conditions of south Western Siberia is investigated. The longwave IR radiative fluxes are calculated on the basis of upper-air sounding data of meteorological station in Novosibirsk for 10 years. The maximum of absolute value of the CO2 radiative forcing was observed at the top of troposphere, at that, in summer, it was higher by 50% than in winter conditions, and relation of CH4 radiative forcing to CO2 forcing at this altitude was about 12%. The sign of the forcing is negative, which means heating of the troposphere. At the top and bottom of the atmosphere, a decrease in CO2 and CH4 radiative forcing is observed with an increase in atmospheric water vapor content, which is caused by overlapping of H2O bands and continuum absorption with CO2 and CH4 absorption bands. The contribution of H2O continuum absorption to the CO2 radiative forcing increases from 30 to 70% when the water vapor atmospheric total column increases from 1 to 4 g/cm2. For winter cases with low water vapor content, the average CO2 radiative forcing at the bottom of the atmosphere increases by 1.5 times in comparison with summer conditions, which leads to additional warming of the surface.

Keywords:

carbon dioxide, methane, water vapor, atmospheric radiative forcing, IR radiation flux

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