Vol. 39, issue 06, article # 1

Gubanova D. P. Natural and anthropogenic impacts on physicochemical characteristics of atmospheric aerosol in the Moscow agglomeration. // Optika Atmosfery i Okeana. 2026. V. 39. No. 06. P. 459–468. DOI: 10.15372/AOO20260601 [in Russian].
Copy the reference to clipboard

Abstract:

The intense urbanization observed in the world is accompanied by the active growth of urban agglomerations. The largest Moscow agglomeration in Europe is currently dynamically developing, which leads to the emergence of additional factors contributing to changes in urban ecosystems, weather and climate. One of the indicators of such processes is the variability of the properties of atmospheric aerosols. In this study, the main types of natural and anthropogenic impacts and their characteristic features are identified. To this end, a comprehensive algorithm for assessing the indicators of typical aerosol pollution of the city atmosphere and classifying impacts has been developed based on the results of continuous six-year (2020–2025) experimental observations at IAP RAS and measurements from the Mosecomonitoring network. The results can be used to clarify the aerosol emissions in Moscow, in chemical transport models, and in assessing and forecasting the state of urban ecosystems and climate.

Keywords:

atmospheric aerosol, РM10, PM2.5, mass concentration, algorithm, conditional background aerosol pollution, natural and anthropogenic impacts, typification, Moscow agglomeration

Figures:

References:

1. Kondrat'ev K.Ya., Ivlev L.S., Krapivin V.F. Atmosfernye aerozoli: Svoistva, protsessy obrazovaniya i vozdeistviya. Ot nano- do global'nykh masshtabov. SPb.: VVMb, 2007. 858 p.
2. Seinfeld J.H., Pandis S.N. Atmospheric Chemistry and Physics: From Air Pollution to Climate Change. New York: Wiley, USA, 2006. 1232 p.
3. Lokoshchenko M.A., Alekseeva L.I. Influence of meteorological parameters on the urban heat island in Moscow // Atmosphere. 2023. V. 14, 507. DOI: 10.3390/atmos14030507.
4. Lokoshchenko M.A. Urban heat island and urban dry island in Moscow and their centennial changes // J. Appl. Meteorol. Climatol. 2017. V. 56. P. 2729-2745. DOI: 10.1175/JAMC-D-16-0383.1.
5. Kuznetsova I.N., Brusova N.E., Nakhaev M.I. Gorodskoi ostrov tepla v Moskve: opredelenie, granitsy, izmenchivost' // Meteorologiya i gidrologiya. 2017. N 5. P. 49–61.
6. Han J.Y., Baik J.J., Lee H. Urban impacts on precipitation // Asia–Pac. J. Atmospheric. Sci. 2014. V. 50. N 1. P. 17–30. DOI: 10.1007/s13143-014-0016-7.
7. Liu J., Niyogi D. Meta-analysis of urbanization impact on rainfall modification // Sci. Rep. 2019. V. 9. P. 7301. DOI: 10.1038/s41598-019-42494-2.
8. Chapman S., Watson J.E.M., Salazar A., Thatcher M., McAlpine C.A. The impact of urbanization and climate change on urban temperatures: A systematic review // Landscape Ecol. 2017. V. 32. P. 1921–1935. DOI: 10.1007/s10980-017-0561-4.
9. Ginzburg A.S., Dokukin S.A. Vliyanie teplovogo zagryazneniya atmosfery na klimat goroda (otsenki s pomoshch'yu modeli COSMO-CLM) // Izv. RAN. Fizika atmosf. i okeana. 2021. V. 57, N 1. P. 53–66. DOI: 10.31857/S0002351521010053.
10. Garuma G. Review of urban surface parameterizations for numerical climate models // Urban Clim. 2018. V. 24. P. 830–851. DOI: 10.1016/j.uclim.2017.10.006.
11. Tarasova M.A., Varentsov M.I., Stepanenko V.M. Parametrizatsii vzaimodeistviya atmosfery s gorodskoi poverkhnost'yu: obzor i perspektivy razvitiya // Izv. RAN. Fizika atmosf. i okeana. 2023. V. 59, N 2. P. 127–148. DOI: 10.31857/S0002351523020062.
12. Han W., Li Z., Guo J., Su T., Chen T., Wei J., Cribb M. The urban–rural heterogeneity of air pollution in 35 metropolitan regions across China // Remote Sens. 2020. V. 12. Р 2320. DOI: 10.3390/rs12142320.
13. Kang L., Chen S., Huang J., Zhao S., Ma X., Yuan T., Zhang X., Xie T. The spatial and temporal distributions of absorbing aerosols over East Asia // Remote Sens. 2017. V. 9. Р 1050. DOI: 10.3390/rs9101050.
14. Doklad «O sostoyanii okruzhayushchei sredy v gorode Moskve v 2022 year» / pod red. A.O. Kul'bachevskogo. M., 2023. 276 p.
15. Popovicheva O., Diapouli E., Chichaeva M., Kosheleva N., Kovach R., Bitukova V., Eleftheriadis K., Kasimov N. Aerosol characterization and peculiarities of source apportionment in Moscow, the largest and northernmost European megacity // Sci. Total Environ. 2024. V. 918. Р. 170315. DOI: 10.1016/j.scitotenv.2024.170315.
16. Elansky N.F., Shilkin A.V., Ponomarev N.A., Semutnikova E.G., Zakharova P.V. Weekly patterns and weekend effects of air pollution in the Moscow megacity // Atmos. Environ. 2020. V. 224. P. 117303. DOI: 10.1016/j.atmosenv.2020.117303.
17. Elansky N.F., Shilkin A.V., Ponomarev N.A., Zakharova P.V., Kachko M.D., Polyakov T.I. Prostranstvenno-vremennye variatsii soderzhaniya zagryaznyayushchikh primesei v vozdushnom basseine Moskvy i ikh emissii // Izv. RAN. Fizika atmosf. i okeana. 2022. V. 58, N 1. P. 92–108. DOI: 10.31857/S0002351522010023.
18. Chubarova N., Androsova E., Kirsanov A., Varentsov M., Rivin G. Urban aerosol, its radiative and temperature response in comparison with urban canopy effects in megacity based on COSMO-ART modeling // Urban Clim. 2024. V. 53. P. 101762. DOI: 10.1016/j.uclim.2023.101762.
19. Chubarova N.E., Vogel H., Androsova E.E., Kirsanov A.A., Popovicheva O.B., Vogel B., Rivin G.S. Columnar and surface urban aerosol in the Moscow megacity according to measurements and simulations with the COSMO-ART model // Atmos. Chem. Phys. 2022. V. 22. P. 10443–10466. DOI: 10.5194/acp-22-10443-2022.
20. Piskunova D., Chubarova N., Poliukhov A., Zhdanova E. Radiative regime according to the new RAD-MSU(BSRN) Complex in Moscow: The roles of aerosol, surface albedo, and sunshine duration //Atmosphere. 2024. V. 15. P. 144. DOI: 10.3390/atmos15020144.
21. Vinogradova A.A., Gubanova D.P., Ivanova Yu.A. Urban contribution to aerosol pollution of the atmospheric surface layer in the Moscow agglomeration // Izv. Atmos. Ocean. Phys. 2026. V. 62, No. 2. P. 263–282. DOI: 10.1134/S0001433826700386.
22. Gubanova D.P., Vinogradova A.A., Lezina E.A., Iordanskii M.A., Isakov A.A. Uslovno-fonovyi uroven' aerozol'nogo zagryazneniya prizemnogo vozdukha v Moskve i prigorode: sezonnye variatsii // Izv. RAN. Fizika atmosf. i okeana. 2023. V. 59, N 6. P. 754–773. DOI: 10.31857/S0002351523060056.
23. Stein A.F., Draxler R.R., Rolph G.D., Stunder B.J.B., Cohen M.D., Ngan F. NOAA's HYSPLIT atmospheric transport and dispersion modeling system // Bull. Am. Meteorol. Soc. 2015. V. 96. P. 2059–2077. DOI: 10.1175/BAMS-D-14-00110.1.
24. Gelaro R., McCarty W., Suárez M.J., Todling R., Molod A., Takacs L., Randles C., Darmenov A., Bosilovich M.G., Reichle R., Wargan K., Coy L., Cullather R., Draper C., Akella S., Buchard V., Conaty A., da Silva A., Gu W., Kim G.K., Koster R., Lucchesi R., Merkova D., Nielsen J.E., Partyka G., Pawson S., Putman W., Rienecker M., Schubert S.D., Sienkiewicz M., ZHao B. The modern-era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) // J. Clim. 2017. V. 30, N 13. P. 5419–5454. DOI: 10.1175/JCLI-D-16-0758.1.
25. Gubanova D.P., Vinogradova A.A., Skorokhod A.I., Iordanskii M.A. Anomal'noe aerozol'noe zagryaznenie vozdukha v Moskve vblizi lokal'nogo antropogennogo istochnika v iyule 2021 year // Gidrometeorologicheskie issledovaniya i prognozy. 2021. N 4. P. 133–147. DOI: 10.37162/2618-9631-2021-4-133-147.
26. Gubanova D.P., Ginzburg A.S., Vinogradova A.A., Chkhetiani O.G., Semenov V.A. Effekt «pyl'noi mgly» v atmosfere megapolisa // Doklady RAN. Nauki o Zemle. 2025. V. 522, N 1. P. 164–172. DOI: 10.31857/S2686739725050202.
27. Gubanova D., Chkhetiani O., Vinogradova A., Skorokhod A., Iordanskii M. Atmospheric transport of dust aerosol from arid zones to the Moscow region in the fall 2020 // AIMS Geosci. 2022. V. 8, N 2. P. 277-302. DOI: 10.3934/geosci.2022017.
28. Gubanova D.P., Vinogradova A.A., Iordanskii M.A., Skorokhod A.I. Variability of near-surface aerosol composition in Moscow in 2020–2021: Episodes of extreme air pollution of different genesis // Atmosphere. 2022. V. 13, № 4. P. 574–599. DOI: 10.3390/atmos13040574.
29. Kuznetsova I.N., Shalygina I.Yu., Nakhaev M.I., Glazkova A.A., Zakharova P.V., Lezina E.A., Zvyagintsev A.M. Neblagopriyatnye dlya kachestva vozdukha meteorologicheskie faktory // Tr. Gidromettsentra Russia. 2014. N 351. P. 154–172.
31. Kuznetsova I.N., Tkacheva Yu.V., Borisov D.V. Metody prognozirovaniya meteorologicheskikh uslovii, vliyayushchikh na zagryaznenie prizemnogo vozdukha // Meteorologiya i gidrologiya. 2024. N 8. P. 87–103. DOI: 10.52002/0130-2906-2024-8-87-103.
32. Gubanova D.P., Iordanskii M.A., Vinogradova A.A., Belikov I.B., Belousov V.A. Problema vybora znachenii plotnosti chastits dlya chislennoi otsenki massovoi kontsentratsii submikronnogo i mikronnogo aerozolya // Optika atmosf. okeana. 2023. V. 36, N 6. P. 469–481. DOI: 10.15372/AOO20230607; Gubanova D.P., Iordanskii M.A., Vinogradova A.A., Belikov I.B., Belousov V.A. Particle density values for numerical estimation of mass concentration of near-surface submicron and micron aerosol // Atmos. Ocean. Opt. 2023. V. 36, N 6. P. 670–684.