Vol. 35, issue 10, article # 4

Pol'kin V. V., Golobokova L. P., Kruglinsky I. A., Pochyufarov A. O., Sakerin S. M., Khuriganova O. I. Statistical generalization of the characteristics of atmospheric aerosol over the White Sea (expeditions 2003–2021). // Optika Atmosfery i Okeana. 2022. V. 35. No. 10. P. 820–825. DOI: 10.15372/AOO20221004 [in Russian].
Copy the reference to clipboard

Abstract:

The paper presents the results of a statistical generalization of the microphysical characteristics and ionic composition of the aerosol in the atmosphere of the White Sea obtained during the expeditions of 2003–2021. Based on the recalculation of the measurement results using a uniform data filtering algorithm, the total number concentration of particles with a radius of 0.2–5 μm, the volumes of particles of fine and coarse dispersed drive aerosol with a radius of less than and more than 0.5 μm, the distribution function of particles by volume are considered, mass concentrations in the composition were estimated aerosol of eight water-soluble ions Ca2+, Mg2+, Na+, K+, NH4+, NO3, Cl, and SO42–. Spatial inhomogeneities and causes of anomalously high concentrations and ionic composition of the aerosol are analyzed.

Keywords:

White Sea, atmospheric aerosol, microphysical characteristics, ionic composition

Figures:

References:

    1. Park J., Dall’Osto M., Park K., Gim Y., Kang H.J., Jang E., Park K.-T., Park M., Yum S.S., Jung J., Lee B.Y., Yoon Y.J. Shipborne observations reveal contrasting Arctic marine, Arctic terrestrial and Pacific marine aerosol properties // Atmos. Chem. Phys. 2020. V. 20, N 5. P. 5573–5590.
    2. Ferrero L., Sangiorgi G., Perrone M.G., Rizzi C., Cataldi M., Markuszewski P., Pakszys P., Makuch P., Petelski T., Becagli S., Traversi R., Bolzacchini E., Zielinski T. Chemical composition of aerosol over the Arctic Ocean from summer ARcticEXpedition (AREX) 2011–2012 cruises: Ions, amines, elemental carbon, organic matter, polycyclic aromatichydrocarbons, n–alkanes, metals, and rare Earth elements // Atmosphere. 2019. V. 10, N 54. DOI: 10.3390/atmos10020054.
    3. Schevchenko V.P., Kopeikin V.M., Evangeliou N., Lisitzin A.P., Novigatsky A.N., Pankratova N.V., Starodymova D.P., Stohl A., Thomson R. Atmospheric black carbon over the north Atlantic and Russian arctic seas in summer–autumn time // Chemistry for sustainable development. 2016. V. 24. P. 441–446. DOI: 10.15372/KhUR20160402.
    4. Xing J., Bian L., Hu Q., Yu J., Sun C., and Xie Z. Atmospheric black carbon along a cruise path through the Arctic Ocean during the Fifth Chinese Arctic Research Expedition // Atmosphere. V. 2014, N 5. P. 292–306. DOI:10.3390/atmos5020292.
    5. Pol'kin V.V., Panchenko M.V., Golobokova L.P. Ionnyj sostav privodnogo aerozolya Belogo morya v august 2003–2006 years // Optika atmosf. i okeana. 2007. V. 20, N 1. P. 988–1003.
    6. Kozlov V.S., Tikhomirov A.B., Panchenko M.V., Shmargunov V.P., Pol’kin V.V., Sakerin S.M., Lisitzin A.P., Shevchenko V.P. Opticheskie i mikrofizicheskie harakteristiki aerozolya v privodnoj atmosfere Belogo morya po dannym odnovremennyh korabel'nyh i beregovyh izmerenij v august 2006 year // Optika atmosf. i okeana. 2009. V. 22, N 8. P. 767–776; Kozlov V.S., Tikhomirov A.B., Panchenko M.V., Shmargunov V.P., Pol’kin V.V., Sakerin S.M., Lisitzin A.P., Shevchenko V.P. Optical and microphysical parameters of aerosol in the near-water atmosphere of the White Sea as assessed from the data of simultaneous ship-borne and coast-based measurements in August 2006 // Atmos. Ocean. Opt. 2009. V. 22, N 5. P. 517–526.
    7. Pol'kin V.V., Golobokova L.P., Pogodaeva T.V., Kozlov V.S., Korobov V.B., Lisitsyn A.P., Panchenko M.V., Peskova M.A., Hodzher T.V., Shevchenko V.P. Sostav aerozolej privodnogo sloya atmosfery nad Belym morem vo vtoroj polovine avgusta 2003 i 2004 years // Fundamental'nye issledovaniya okeanov i morej. N.P. Laverov (red.). M.: Nauka, 2006. P. 413–439.
    8. Pol'kin V.V., Panchenko M.V., Golobokova L.P., Filippova U.G., Hodzher T.V., Lisitsyn A.P., Shevchenko V.P. Privodnyj aerozol' Belogo i Karskogo morej v august–september 2007 year // Meteorologicheskie i geofizicheskie issledovaniya. М.: Paulsen, 2011. P. 199–214.
    9. Turchinovich Yu.S., Pochufarov A.O., Sakerin S.M. Algorithm of controlling the quality and retrieval of data from measurements of aerosol and black carbon concentrations in marine expeditions // Proc. SPIE. 2021. V. 11916. 119161U [11916-20]. DOI: 10.1117/12.2600591.
    10. Shmargunov V.P., Pol'kin V.V. Aerozol'nyj schetchik na baze AZ-5. // Pribory i tekhnika eksperimenta. 2007. N 2. P. 65.
    11. Schetchik aerozol'nyh chastits АЗ-10-0. URL: https://eco-intech.com/product/schetchik-chastits-az-10 (data obrashcheniya: 06.05.2022).
    12. Kozlov V.S., Shmargunov V.P., Panchenko M.V. Modified aethalometer for monitoring of black carbon concentration in atmospheric aerosol and technique for correction of the spot loading effect // Proc. SPIE. 2016, 1003530. DOI: 10.1117/12.2248009.
    13. Petzold A., Ogren J.A., Fiebig M., Laj P., Li S.-M., Baltensperger U., Holzer-Popp T., Kinne S., Pappalardo G., Sugimoto N., Wehrli C., Wiedensohler A., and Zhang X.-Y. Recommendations for reporting “black carbon” measurements // Atmos. Chem. Phys. 2013. V. 13. P. 8365–8379. DOI: 10.5194/acp-13-8365-2013.
    14. Golobokova L.P., Hodzher T.V., Chernov D.G., Sidorova O.R., Huriganova O.I., Onishchuk N.A., ZHuchenko N.A., Marinajte I.I. Himicheskij sostav prizemnogo atmosfernogo aerozolya v Barentsburge arhipelag Shpitsbergen) po rezul'tatam mnogoletnih issledovanij // Lyod i cneg. 2020. V. 60, N 1. P. 85–97. DOI: 10.31857/S2076673420010025.
    15. Pol'kin V.V., Shchelkanov N.N., Golobokova L.P., Panchenko M.V. Sravnenie metodik otsenki vklada kontinental'nyh i morskih istochnikov v ionnyj sostav privodnogo aerozolya Belogo morya // Optika atmosf. i okeana. 2008. V. 21, N 1. P. 23–26.
    16. Millero F.J. Chemical Oceanography. 4th ed. Boca Raton: CRC Press, Florida: 2016. 591 p.
    17. Air Resources Laboratory – HYSPLIT, Modified April 1, 2020, https://ready.arl.noaa.gov/HYSPLIT.php (last access February 2022).
    18. Giovanni: The Bridge between Data and Science v 4.35. https://giovanni.gsfc.nasa.gov/giovanni (last access February 2022).
    19. Pol'kin V.V., Golobokova L.P., Kruglinskij I.A., Pochufarov A.O., Sakerin S.M., Huriganova O.I. Statisticheskoe obobshchenie harakteristik atmosfernogo aerozolya nad Belym morem: ekspeditsii 2003–2021 years // Optika atmosfery i okeana. Fizika atmosfery: Materialy XXVIII Mezhdunar. simpoz., g. Tomsk, 4–8 july 2022 year. – Tomsk: Izd-vo IOA SO RAN, 2022. – 1 elektron. opt. disk (CD-ROM). P. C23-C28. ISBN 978-5-94458-190-7.
    20. Sakerin S.M., Golobokova L.P., Kabanov D.M., Kozlov V.S., Pol’kin V.V., Radionov V.F., Chernov D.G. Sravnenie srednih harakteristik aerozolya v sosednih arkticheskih rajonah // Optika atmosf. i okeana. 2018. V. 31, N 8. P. 640–646; Sakerin S.M., Golobokova L.P., Kabanov D.M., Kozlov V.S., Pol’kin V.V., Radionov V.F., Chernov D.G. Comparison of average aerosol characteristics in neighboring Arctic regions // Atmos. Ocean. Opt. 2019. V. 32, N 1. P. 33–40.
    21. Sakerin S.M., Kabanov D.M., Makarov V.I., Polkin V.V., Popova S.A., Chankina O.V., Pochufarov A.O., Radionov V.F., Rize D.D. Spatial distribution of atmospheric aerosol physicochemical characteristics in Russian sector of the Arctic Ocean // Atmosphere. 2020. V. 11, N 11. P. 1170. DOI: 10.3390/atmos11111170.
    22. Tsellyulozno-bumazhnoe proizvodstvo / Tekhnologiya i oborudovanie lesohimicheskih proizvodstv. [Elektronnyj resurs]. http://msd.com.ua.